I messed around with enriching the carbon dioxide for a while, using a controller that was on for “so many” seconds, “so many” times per minute - the latter being the adjusted setting for concentration.
Level testing was a premade glass tube with a premixed reagent that changed color once opened and left exposed to the atmosphere for a few minutes.
I was attempting this in a 14’ x 18’, “well sealed” greenhouse. It wasn’t, as it turned out, so that made keeping the level up was a super challenge, as was hauling around the gas cylinders and paying for them.
I did manage to achieve 1500 ppm for about 3 months and saw no discernible change in anything but my bank account.